4.8 Article

Thermopower and Unconventional Nernst Effect in the Predicted Type-II Weyl Semimetal WTe2

Journal

NANO LETTERS
Volume 18, Issue 10, Pages 6591-6596

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.8b03212

Keywords

Transition Metal Dichalcogenide; WTe2; Weyl semimetal; Nernst effect; 2D material; Thermopower

Funding

  1. ERC [670166, 742068]
  2. European Research Council (ERC) [670166] Funding Source: European Research Council (ERC)

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WTe2 is one of a series of recently discovered high mobility semimetals, some of whose properties are characteristic of topological Dirac or Weyl metals. One of its most interesting properties is the unsaturated giant magnetoresistance that it exhibits at low temperatures. An important question is the degree to which this property can be ascribed to a conventional semimetallic model in which a highly compensated, high mobility metal exhibits large magnetoresistance. Here, we show that the longitudinal thermopower (Seebeck effect) of semimetallic WTe2 exfoliated flakes exhibits periodic sign changes about zero with increasing magnetic field that indicates distinct electron and hole Landau levels and nearly fully compensated electron and hole carrier densities. However, inconsistent with a conventional semimetallic picture, we find a rapid enhancement of the Nernst effect at low temperatures that is nonlinear in magnetic field, which is consistent with Weyl points in proximity to the Fermi energy. Hence, we demonstrate the role played by the Weyl character of WTe2 in its transport properties.

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