4.8 Article

Chemical Vapor Deposition of Thin Crystals of Layered Semiconductor SnS2 for Fast Photodetection Application

Journal

NANO LETTERS
Volume 15, Issue 1, Pages 506-513

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/nl503857r

Keywords

Layered semiconductor; metal dischalcogenide; chemical vapor deposition; low-dimensional materials; single-crystal arrays

Funding

  1. National Science Foundation [ECCS-1247874]
  2. State of Texas through the Texas Center for Superconductivity (TcSUH) at the University of Houston
  3. Robert A. Welch Foundation [E-1146]

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Layered two-dimensional (2D) semiconductors, such as MoS2 and SnS2, have been receiving intensive attention due to their technological importance for the next-generation electronic/photonic applications. We report a novel approach to the controlled synthesis of thin crystal arrays of SnS2 at predefined locations on chip by chemical vapor deposition with seed engineering and have demonstrated their application as fast photodetectors with photocurrent response time similar to 5 mu s. This opens a pathway for the large-scale production of layered 2D semiconductor devices, important for applications in integrated nanoelectronic/photonic systems.

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