4.8 Article

Room-Temperature Near-Infrared High-Q Perovskite Whispering-Gallery Planar Nano lasers

Journal

NANO LETTERS
Volume 14, Issue 10, Pages 5995-6001

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/nl503057g

Keywords

Organic-inorganic perovskites; whispering gallery mode lasing; near-infrared lasers; nanoplatelets; wavelength tunable; on-chip integration

Funding

  1. Singapore Ministry of Education [MOE2011-T2-2-051]
  2. Singapore National Research Foundation [NRF-RF2009-06]
  3. Competitive Research Program [NRF-CRP-6-2010-2, NRF-CRP5-2009-04]
  4. Nanyang Technological University [M58110061]
  5. New Initiative Fund [M58110100]
  6. NTU [M4080514]
  7. SPMS collaborative Research [M4080536]
  8. Ministry of Education [M0E2013-T2-1-081]
  9. National Research Foundation (NRF), Prime Minister's Office, Singapore under its Campus for Research Excellence and Technological Enterprise (CREATE) programme

Ask authors/readers for more resources

Near-infrared (NIR) solid state micro/nanolasers are improtant building blocks for true integration of optoelectronic circuitry.(1) Although significant progress has been made in III-V nanowire lasers with achieving NIR lasing at room temperature,(2-4) challenges remain including low quantum efficiencies and high auger losses. Imporatntly, the obstacles toward integrating one-dimensioanl nanowires on the planar ubquitous Si platform need to be effectively tackled. Here we demonstrate a new family of planar room-temperature NIR nanolasers based on organic-inorganic perovskite CH3NH3PbI3-aXa (X = I, Br, Cl) nanoplatelets. Their large exciton binding energies, long diffusion lengths, and naturally formed high quality planar whispering-gallery mode cavities ensure adequate gain and efficient optical feedback for low-threshold optically pumpbed in-plane lasing. We show that these remarkable wavelength tunable whispering-gallery nanolasers can be easily integrated onto conductive platforms (Si, Au, indium tin oxidie, and so forth). Our findings open up a new class of wavelength tunable palanar nanomaterials potentially suitable for on-chip integration.

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