4.8 Article

An Advanced Lithium-Ion Battery Based on a Graphene Anode and a Lithium Iron Phosphate Cathode

Journal

NANO LETTERS
Volume 14, Issue 8, Pages 4901-4906

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/nl502429m

Keywords

Graphene; nanoflakes; inks; anode; lithium ion battery

Funding

  1. Graphene Flagship [CNECT-ICT-604391]
  2. Lancaster University through the Distinguished Visitor Programme in Physical Sciences

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We report an advanced lithium-ion battery based on a graphene ink anode and a lithium iron phosphate cathode. By carefully balancing the cell composition and suppressing the initial irreversible capacity of the anode in the round of few cycles, we demonstrate an optimal battery performance in terms of specific capacity, that is, 165 mAhg(-1), of an estimated energy density of about 190 Wh kg(-1) and a stable operation for over 80 charge-discharge cycles. The components of the battery are low cost and potentially scalable. To the best of our knowledge, complete, graphene-based, lithium ion batteries having performances comparable with those offered by the present technology are rarely reported; hence, we believe that the results disclosed in this work may open up new opportunities for exploiting graphene in the lithium-ion battery science and development.

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