Journal
NANO LETTERS
Volume 14, Issue 6, Pages 3191-3196Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nl500524w
Keywords
Single-molecule magnets; molecular spintronics; Franck-Condon blockade; electron-vibron coupling
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Funding
- EU
- advanced ERC Grant (Mols@Mols)
- Dutch funding organization NWO (VENI)
- OCW
- U.S. National Science Foundation [DMR-0804665, DMR-1206354, DMR060009N]
- [618082 ACMOL]
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [1206354] Funding Source: National Science Foundation
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We investigate vibron-assisted electron transport in single-molecule transistors containing an individual Fe-4 Single-Molecule Magnet. We observe a strong suppression of the tunneling current at low bias in combination with vibron-assisted excitations. The observed features are explained by a strong electron-vibron coupling in the framework of the Franck-Condon model supported by density-functional theory.
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