4.8 Article

Transport Studies of Dual-Gated ABC and ABA Trilayer Graphene: Band Gap Opening and Band Structure Tuning in Very Large Perpendicular Electric Fields

Journal

NANO LETTERS
Volume 13, Issue 2, Pages 369-373

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/nl303375a

Keywords

Trilayer graphene; stacking dependence; electrical transport; tunable band gap; two-band transport; self-consistent Hartree screening

Funding

  1. ONR [N00014-11-1-0730]
  2. DARPA [SPAWAR N66001-11-1-4110]
  3. NNIN REU
  4. Welch Foundation [TBF1473]
  5. DOE Division of Materials Sciences and Engineering [DE-FG03-02ER45958]
  6. Direct For Mathematical & Physical Scien
  7. Division Of Materials Research [0959764] Funding Source: National Science Foundation

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We report on the transport properties of ABC and ABA stacked trilayer graphene using dual, locally gated field effect devices. The high efficiency and large breakdown voltage of the HfO2 top and bottom gates enable independent tuning of the perpendicular electric field and the Fermi level over an unprecedentedly large range. We observe a resistance change of 6 orders of magnitude in the ABC trilayer, which demonstrates the opening of a band gap. Our data suggest that the gap saturates at a large displacement field of D similar to 3 V/nm, in agreement with self-consistent Hartree calculations. In contrast, the ABA trilayer remains metallic even under a large perpendicular electric field. Despite the absence of a band gap, the band structure of the ABA trilayer continues to evolve with increasing D. We observe signatures of two-band conduction at large D fields. Our self-consistent Hartree calculation reproduces many aspects of the experimental data but also points to the need for more sophisticated theory.

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