Journal
NANO LETTERS
Volume 11, Issue 9, Pages 3557-3563Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nl201004c
Keywords
Nanocavities; plasmonics; nanoimprint; perfect absorbers; LSPR resonances; refractive index sensing
Categories
Funding
- TERAMAGSTOR
- ULTRACIS
- METAPHOTONIQUE ANR
- PRF Metamat ONERA
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Arrays of plasmonic nanocavities with very low volumes, down to lambda(3)/1000, have been fabricated by soft UV nanoimprint lithography. Nearly perfect omnidirectional absorption (3-70 degrees) is demonstrated for the fundamental mode of the cavity (lambda similar or equal to 1.15 mu m). The second-order mode exhibits a sharper resonance with strong angular dependence and total optical absorption when the critical coupling condition is fulfilled (45-50 degrees, lambda similar or equal to 750 nm). It leads to high refractive index sensitivity (405 nm/RIU) and figure of merit (similar to 21) and offers new perspectives for efficient biosensing experiments in ultralow volumes.
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