Journal
NANO LETTERS
Volume 10, Issue 5, Pages 1717-1721Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nl1000949
Keywords
Single nanoparticle; gold; plasmonics; nonlinear optics; second harmonic generation; finite element method simulation
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We report the optical second harmonic generation from individual 150 nm diameter gold nanoparticles dispersed in gelatin. The quadratic hyperpolarizability of the particles is determined and the input polarization dependence of the second harmonic intensity obtained. These results are found in excellent agreement with ensemble measurements and finite element simulations. These results open up new perspectives for the investigation of the nonlinear optical properties of noble metal nanoparticles.
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