Journal
NANO LETTERS
Volume 10, Issue 10, Pages 3995-3999Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nl1018639
Keywords
Quantum dot; J-aggregate; energy transfer; electrostatic; thin film
Categories
Funding
- National Science Foundation
- DOE Basic Energy Sciences [DE-FG02-07ER46454]
- Chesonis Family Foundation
- ISN [W911NF-07-D-0004]
- NSF-MRSEC [DMR-0819762]
- U.S. Department of Energy (DOE) [DE-FG02-07ER46454] Funding Source: U.S. Department of Energy (DOE)
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [0819762, GRANTS:13714308] Funding Source: National Science Foundation
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This paper describes the solution preparation of thin films composed of quantum dots and thiacyanine J-aggregates, making use of the size tunable emission of quantum dots and the narrow, intense absorption off-aggregates in the solid state These blended films exhibit 90% energy transfer efficiency from J-aggregates to quantum dots and can uniformly cover a large area Because the presence of chef-aggregates enhances the QD photoluminescence intensity by 2 5-fold over QDs alone, these solid state materials may be useful in downconversion applications or in fundamental investigations of light harvesting
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