Journal
NANO LETTERS
Volume 9, Issue 11, Pages 3909-3913Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nl9021094
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- Zernike Institute for Advanced Materials
- Nederlandse Organisatie voor Wetenschappelijk onderzoek, NWO
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The promise of transition voltage spectroscopy (TVs) is that molecular level positions can be determined in molecular devices without applying extreme voltages. Here, we consider the physics behind TVs in more detail. Remarkably, we find that the Simmons model employed thus far is inconsistent with experimental data. However, a coherent molecular transport model does justify TVS as a spectroscopic tool. Moreover, TVS may become a critical test to distinguish molecular junctions from vacuum tunnel junctions.
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