Journal
NANO LETTERS
Volume 9, Issue 6, Pages 2477-2481Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nl901253t
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Funding
- DFG [SFB 448]
- Rede Nanofoton/CNPq (Brazilian agency)
- Alexander von Humboldt Foundation
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In this Letter we report on the investigation of the upconversion emission of single NaYF4 nanocrystals codoped with Yb3+ and Er3+. Single nanocrystals on a coverslip are excited with continuous wave laser light at 973 nm in a confocal setup and the upconversion fluorescence is analyzed with a spectrometer. With the help of an atomic force microscope the size of the nanocrystals is simultaneously determined. A strong size-dependence of the spectral properties of the upconversion signal of individual nanocrystals is observed. We attribute this to a differing number of available phonons in the individual crystals for multiphonon relaxation processes, depending on their size. We believe that this result provides a new strategy in the synthesis of upconversion nanoparticles with different spectral properties by changing only their size as it is well-known from the case of semiconductor quantum dots.
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