4.8 Article

Plasmon Dispersion in Coaxial Waveguides from Single-Cavity Optical Transmission Measurements

Journal

NANO LETTERS
Volume 9, Issue 8, Pages 2832-2837

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/nl900597z

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Funding

  1. National Science Foundation [DMR 0606472]
  2. Center for Science and Engineering of Materials
  3. Stichting voor Fundamenteel Onderzoek der Materie (FOM)
  4. Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO)
  5. Dutch Ministry of Economic Affairs

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We determine the plasmon dispersion relation in coaxial waveguides composed of a circular channel separating a metallic core and cladding. Optical transmission measurements are performed on isolated coaxial nanoapertures fabricated on a Ag film using focused ion-beam lithography. The dispersion depends strongly on the dielectric material and layer thickness. Our experimental results agree well with an analytical model for plasmon dispersion in coaxial waveguides. We observe large phase shifts at reflection from the end facets of the coaxial cavity, which strongly affect the waveguide resonances and can be tuned by changing the coax geometry, composition, and surrounding dielectric index, enabling coaxial cavities with ultrasmall mode volumes.

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