Journal
NANO LETTERS
Volume 9, Issue 2, Pages 655-658Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nl802998e
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- U.S. Department of Energy Office of Basic Energy [DE-AC06-RL01830]
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Here we report that clay nanoparticles allow formation of a modified transparent electrode, spontaneous adsorption of fluorescent redox molecules on the clay layer, and thus the subsequent observation of single-molecule fluorescence spectroelectrochemistry. We can trace single-molecule fluorescence spectroelectrochemistry by probing the fluorescence intensity change of individually immobilized single redox molecules modulated via cyclic voltammetric potential scanning. This work opens a new approach to explore interfacial electron transfer mechanisms of redox reactions.
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