Journal
MOLECULAR PHYSICS
Volume 108, Issue 11, Pages 1415-1433Publisher
TAYLOR & FRANCIS LTD
DOI: 10.1080/00268971003762134
Keywords
x-ray and neutron scattering; x-ray absorption and emission spectroscopy; mixture and continuum models; empirical and ab initio theory
Funding
- NSF
- Department of Energy
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We review the spectroscopic techniques and scattering experiments used to probe the structure of water, and their interpretation using empirical and ab initio models, over the last 5 years. We show that all available scientific evidence overwhelmingly favors the view of classifying water near ambient conditions as a uniform, continuous tetrahedral liquid. While there are controversial issues in our understanding of water in the supercooled state, in confinement, at interfaces, or in solution, there is no real controversy in what is understood as regards bulk liquid water under ambient conditions.
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