Journal
MACROMOLECULES
Volume 45, Issue 5, Pages 2509-2513Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ma3002092
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Funding
- BU
- Advanced Energy Consortium
- NIH [GM27278]
- NSF [CHE-1012464]
- Conseil general d'Aquitaine
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [1012464] Funding Source: National Science Foundation
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A polystyrenylphosphonium polymer was synthesized and complexed with various carboxylic acid derivatives to form new solid-state polyelectrolyte-surfactant assemblies. The properties of these ionic materials were highly dependent on the nature of the anion and included a brittle material, a rubbery ball that bounces, or a sticky fiber. The values for the equilibrium modulus, storage modulus, and loss modulus were dependent on the composition of the carboxylic acid and the number of electrostatic interactions. Small-angle X-ray scattering studies on the supramolecular assemblies confirmed a bilayer structure for two of the assemblies.
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