Journal
MACROMOLECULAR CHEMISTRY AND PHYSICS
Volume 210, Issue 24, Pages 2160-2166Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/macp.200900346
Keywords
copolymerization; hydrophilic polymers; molecular dynamics
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Funding
- Ministry of Education, Culture, Sports, Science and Technology, Japan
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The behavior of the transmittance self-oscillation of a polymer chain with a positively charged MAPTAC group is studied. The polymer concentration exerts considerable influence on the behavior and lifetime of the self-oscillation. The redox potential and transmittance are measured simultaneously showing that the reactivity of the Ru(bpy)(3) moiety is significantly affected by the polymer aggregation state, originating from the solubility of the polymer chain. The behavior and lifetime of the self-oscillation can be controlled by changing the design of the polymer structure and concentration.
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