Journal
LASER PHYSICS
Volume 19, Issue 8, Pages 1691-1696Publisher
IOP PUBLISHING LTD
DOI: 10.1134/S1054660X0915047X
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Funding
- National Natural Science Foundation of China [10534010, 10634020, 10821062]
- National Basic Research Program of China [2006CB806007]
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Field-free molecular alignment can be achieved by nonadiabatic rotational excitation of molecules with strong femtosecond laser pulses. We experimentally and theoretically demonstrate that the degree of alignment can be improved with multi-pulse excitation. An approach is proposed to tune the frequency of few-cycle pulses using field-free alignment of molecules.
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