Journal
LANGMUIR
Volume 29, Issue 3, Pages 957-964Publisher
AMER CHEMICAL SOC
DOI: 10.1021/la303663x
Keywords
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Funding
- Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry
- National Natural Science Foundation of China [21101014, 21273022, 21073018]
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As advanced electrodes for direct alcohol fuel cells, graphene-Pd and graphene-Pt composites with a trace of SnO2 have been successfully synthesized by a modified electroless plating technique. The surface of graphene oxide is first sensitized by Sn2+ ions, and subsequently, Pd or Pt nanoparticles are deposited on the surface of graphene oxide. Finally, graphene oxide was reduced to graphene by further adding NaBH4. Compared to other carbon-(e.g., Vulcan XC-72R) supported Pd and Pt, the resultant graphene-Pd and Pt composites exhibit better electrocatalytic activity and long-term stability toward alcohol electrooxidation. Additionally, a trace amount of SnO2 formed around active catalysts may also be beneficial to the enhancement of electrochemical activity.
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