4.3 Article

Structural Quantum Criticality and Superconductivity in Iron-Based Superconductor Ba(Fe1-xCox)2As2

Journal

JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN
Volume 81, Issue 2, Pages -

Publisher

PHYSICAL SOC JAPAN
DOI: 10.1143/JPSJ.81.024604

Keywords

iron-based superconductor; elastic constant; quantum criticality; electron-lattice coupling

Funding

  1. Ministry of Education, Culture, Sports, Science and Technology, Japan [20102007]
  2. Japan Science and Technology Agency
  3. Grants-in-Aid for Scientific Research [24540354, 10J56172, 20102005, 20102007, 22540380, 22654037] Funding Source: KAKEN

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We investigated the elastic properties of the iron-based superconductor Ba(Fe1-xCox)(2)As-2 with eight Co concentrations. The elastic constant C-66 shows a large elastic softening associated with structural phase transition. C66 was analyzed on the basis of the localized and itinerant pictures of Fe-3d electrons, which shows a strong electron-lattice coupling and a possible mass enhancement in this system. The results are similar to those of unconventional superconductors, where the properties of the system are governed by quantum fluctuations associated with the zero-temperature critical point of long-range order, namely, the quantum critical point (QCP). In this system, the inverse of C-66 behaves just like the magnetic susceptibility in magnetic QCP systems. Although the QCPs of these existing superconductors are all ascribed to antiferromagnetism, our systematic studies on the canonical iron-based superconductor Ba(Fe1-xCox)(2)As-2 have revealed that there is a signature of structural quantum criticality in this material, which thus far has had no precedent. The elastic constant anomaly is suggested to concern with the emergence of superconductivity. These results highlight the strong electron-lattice coupling and effect of the band in this system, thus challenging the prevailing scenarios that focus on the role of iron 3d orbitals.

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