4.3 Article

Electronic structure and electron correlation in LaFeAsO1-xFx and LaFePO1-xFx

Journal

JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN
Volume 77, Issue 9, Pages -

Publisher

PHYSICAL SOC JAPAN
DOI: 10.1143/JPSJ.77.093714

Keywords

LaFeAsO; electronic structure; photoemission spectroscopy

Funding

  1. Ministry of Education, Culture. Sports, Science and Technology (MEXT)
  2. CREST, Japan Science and Technology Agency
  3. Photon Factory Program Advisory Committee [2006S2-001]

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Photoemission spectroscopy is used to investigate the electronic structure of the newly discovered iron-based superconductors LaFeAsO1-xFx and LaFePO1-xFx. Line shapes of the Fe 2p core-level spectra suggest an itinerant character of Fe 3d electrons. The valence-band spectra are generally consistent with band-structure calculations except for the shifts of Fe 3d-derived peaks toward the Fermi level. From the spectra taken in the Fe 3p -> 3d core-absorption region, we have obtained the experimental Fe 3d partial density of states, and explained it in terms of a band-structure calculation with a phenomenological self-energy correction, yielding a mass renormalization factor of <= 2.

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