4.4 Article

Role of upconversion in optical refrigeration: A theoretical study of laser cooling with Ho3+ doped fluoride crystals

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OPTICAL SOC AMER
DOI: 10.1364/JOSAB.30.003041

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Funding

  1. Specialized Research Fund for the Program for New Century Excellent Talents in University [NCET-11-269]
  2. National Natural Science Foundation of China [11204048, 61275138, 10804022, 60878016]
  3. Fundamental Research Funds for the Central Universities [HEUCFZ1221, HEUCFZ1217]
  4. Special Financial Grant from the China Postdoctoral Science Foundation [2013T60345]
  5. 111 project to the Harbin Engineering University [B13015]

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We present a generalized model for optical refrigeration with Ho3+ doped fluoride crystals in which the dopant concentration dependent upconversion is considered. Based on the spectrum properties of candidate rare-earth ions (Ho3+, Tm3+, and Er3+) for optical refrigeration, a common criterion for upconversion assisted cooling is derived. The cooling performances of Ho3+:YLiF4 crystals are simulated to reveal the practical dopant concentration range for cooling. It is found that the optimal dopant concentration is determined by a balancing consideration of heat loads induced by background absorption and fluorescence quenching. The appropriate pump wavelengths for optical refrigeration with Ho3+:YLiF4 crystals are also indicated. (C) 2013 Optical Society of America

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