Journal
JOURNAL OF THE IRANIAN CHEMICAL SOCIETY
Volume 15, Issue 12, Pages 2851-2860Publisher
SPRINGER
DOI: 10.1007/s13738-018-1471-3
Keywords
Synthetic methodology; Graphene oxide; Hydroformylation; C-N bond formation; Recyclability
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Funding
- National Natural Science Foundation of China [21402168]
- Scientific Research Foundation of Hunan Provincial Education Department [15B232]
- National Natural Science Foundation of Hunan Province [2018JJ2389]
- Hunan 2011 Collaborative Innovation Center of Chemical Engineering & Technology with Environmental Benignity and Effective Resource Utilization
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Graphene oxide (GO), an inexpensive, environment-friendly, and metal-free carbocatalyst, used for the N-formylation of amines is developed. In this reaction, GO shows good activity, selectivity, and recyclability. This strategy has an array of advantages, such as being metal free, without additive, wide-scope protocol, scalable with a low catalyst loading of 3wt%, use of readily available and recyclable carbocatalyst, and DMF as a readily available formyl source. Furthermore, this strategy provides an avenue for the convenient hydroformylation of various amines. [GRAPHICS]
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