Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 136, Issue 45, Pages 15929-15932Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja510475n
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- Aarhus University
- Carlsberg Foundation
- FNU
- Alma Mater Studiorum-University of Bologna
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The organocatalytic asymmetric alpha-alkylation of aldehydes by 1,6-conjugated addition of enamines to p-quinone methides is described. Employing a newly developed class of chiral secondary amine catalysts, alpha-diarylmethine-substituted aldehydes with two contiguous stereocenters have been synthesized in a simple manner with good diastereocontrol and excellent enantioselectivity.
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