Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 136, Issue 19, Pages 6790-6793Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja5003907
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- JSPS
- AIST
- Grants-in-Aid for Scientific Research [12F02209] Funding Source: KAKEN
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High-surface-area N-decorated nanoporous carbons have been successfully synthesized using the N-rich metal-organic framework ZIF-8 as a template and precursor along with furfuryl alcohol and NH4OH as the secondary carbon and nitrogen sources, respectively. These carbons exhibited remarkable CO2 adsorption capacities and CO2/N-2 and CO2/CH4 selectivities. The N-decoration in these carbons resulted in excellent activity for the oxygen reduction reaction. Samples NC900 and NC1000 having moderate N contents, high surface areas, and large numbers of mesopores favored the four-electron reduction pathway, while sample NC800 having a high N content, a moderate surface area, and a large number of micropores favored the two-electron reduction process.
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