Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 136, Issue 45, Pages 15881-15884Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja5092672
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Funding
- University of Nebraska-Lincoln
- NSF through Nebraska MRSEC [DMR-0820521]
- Divisions of Chemistry (CHE) and Materials Research (DMR), National Science Foundation [NSF/CHE-1346572]
- U.S. DOE [DE-AC02-06CH11357]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [1346572] Funding Source: National Science Foundation
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An anionic indium porphyrin framework (UNLPF-10) consisting of rare Williams b-tetrakaidecahedral cages was constructed using an octatopic ligand linked with 4-connected [In(COO)(4)](-) SBUs. Remarkably, the extent of indium metalation of porphyrin macrocycles in UNLPF-10 can be facilely tuned in situ depending on the M/L ratio during synthesis, resulting in a controllable framework charge density and photocatalytic activity toward the selective oxygenation of sulfides.
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