Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 136, Issue 18, Pages 6598-6601Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja503023h
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Funding
- JSPS KAKENHI [20002004, 25221301]
- Platform for Drug Discovery, Informatics, and Structural Life Science (MEXT)
- Mochida Memorial Foundation for Medical and Pharmaceutical Research
- Uehara Memorial Foundation
- JSPS
- Grants-in-Aid for Scientific Research [12J10970] Funding Source: KAKEN
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The first asymmetric total synthesis of lepenine has been accomplished. The synthesis features a tethered intramolecular Diels-Alder reaction, an intramolecular Mannich reaction, and a Diels-Alder reaction between an ortho-quinone monoketal and ethylene, resulting in stereoselective construction of the unique hexacyclic system.
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