Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 29, Pages 10622-10625Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja405012w
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Funding
- NSFC [91027025, 21225417]
- MOST [2011CB932503, 2011DFA51330]
- STCSM [11520701400, 12nm0503200]
- Fok Ying Tong Education Foundation
- Program for Professor of Special Appointment at Shanghai Institutions of Higher Learning
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An organic thiolate/disulfide redox couple with low absorption in the visible region was developed for use in fabricating novel dye-sensitized photovoltaic wires with an aligned carbon nanotube (CNT) fiber as the counter electrode. These flexible wire devices achieved a maximal energy conversion efficiency of 7.33%, much higher than the value of 5.97% for the conventional I-/I-3(-) redox couple. In addition, the aligned CNT fiber also greatly outperforms the conventional Pt counter electrode with a maximal efficiency of 2.06% based on the thiolate/disulfide redox couple.
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