Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 37, Pages 13934-13938Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja406844r
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Funding
- Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]
- National Natural Science Foundation of China [21371162, 51301159]
- University of Science and Technology of China (USTC)
- NSF [DBI-0116835]
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A reaction between a Zr-IV salt and a porphyrinic tetracarboxylic acid leads to a metal-organic framework (MOF) with two types of open channels, representing a MOF featuring a (4,8)-connected sqc net. The MOF remains intact in both boiling water and aqueous solutions with pH ranging from 1 to 11, a remarkably extensive pH range that a MOF can sustain. Given its exceptional stability and pH-dependent fluorescent intensity, the MOF can potentially be applied in fluorescent sensing.
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