Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 2, Pages 558-561Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja310098k
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Funding
- National Natural Science Foundation of China [21290191, 20952001, 21021091]
- National Major State Basic Research Development Program [2011CB808401, 2011CB932304]
- Chinese Academy of Sciences
- DST, New Delhi [SR/S1/OC-27/2009]
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Fullerene/sulfur-bridged annulene cocrystals with a two-dimensional segregated alternating layer structure were prepared by a simple solution process. Single-crystal analysis revealed the existence of continuing pi-pi interactions in both the donor and acceptor layers, which serve as transport paths for holes and electrons separately. The ambipolar transport behaviors were demonstrated with single-crystal field-effect transistors and rationalized by quantum calculations. Meanwhile, preliminary photoresponsivity was observed with the transistor configuration.
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