Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 43, Pages 16038-16041Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja408508m
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Funding
- Welch Foundation [F-1738]
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MCl2 complexes of a new p-carboxylated 1,2-bis(diphenylphosphino)benzene ligand are effectively utilized as tetratopic building blocks to prepare isostructural porous coordination polymers with accessible reactive metal sites (M = Pd, Pt). The crystalline materials exhibit unusual and fully reversible H-2 sorption at 150 degrees C. Post-synthetic reactivity is also possible, in which Pt-Cl bonds can be activated to provide organometallic species in the pores.
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