Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 136, Issue 2, Pages 626-629Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja411596q
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Funding
- NIHGMS [R01 GM103558-01]
- Carlsberg Foundation
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Direct C-H functionalization and arylation of benzyl ethers has been accomplished via photoredox organocatalysis. The productive merger of a thiol catalyst and a commercially available iridium photoredox catalyst in the presence of household light directly affords benzylic arylation products in good to excellent yield. The utility of this methodology is further demonstrated in direct arylation of 2,5-dihydrofuran to form a single regioisomer.
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