Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 42, Pages 15750-15753Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja4092903
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Funding
- National Basic Research Program of China (973 Program) [2013CB632402, 2011CB921404]
- National Science Foundation of China [21073069, 91023010, 21177048]
- FDA Nanotechnology CORES Program
- Office of Cosmetics and Colors, CFSAN/FDA
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We demonstrate that BiOCl single-crystalline nanosheets possess surface structure-dependent molecular oxygen activation properties under UV light. The (001) surface of BiOCl prefers to reduce O-2 to center dot O-2(-) through one-electron transfer, while the (010) surface favors the formation of O-2(2-) via two-electron transfer, which is cogoverned by the surface atom exposure and the situ generated oxygen vacancy characteristics of the (001) and (010) surfaces under UV light irradiation.
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