Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 14, Pages 5332-5335Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja401840j
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Funding
- Marie Curie Foundation
- Cancer Research UK
- University of Cambridge
- ERC
- EPSRC
- Cancer Research UK [6934] Funding Source: researchfish
- Engineering and Physical Sciences Research Council [EP/I00548X/1] Funding Source: researchfish
- EPSRC [EP/I00548X/1] Funding Source: UKRI
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Copper catalysts enable the electrophilic carbofunctionalization of alkynes with vinyl- and diaryliodonium triflates. The new process forms highly substituted alkenyl triflates from a range of alkynes via a pathway that is opposite to classical carbometalation. The alkenyl triflate products can be elaborated through cross-coupling reactions to generate synthetically useful tetrasubstituted alkenes
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