Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 25, Pages 9475-9479Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja402479r
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Funding
- National Science Foundation [CHE - 1212446]
- Department of Education
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Iron(III)chloride catalyzes the aerobic oxidation of tertiary anilines, including tetrahydroisoquinolines, to form reactive iminium ion intermediates that undergo Mannich reactions with silyloxyfurans, nitroalkanes, and other nucleophiles to give the corresponding butenolides, nitro compounds, and alpha-substituted tetrahydroisoquinolines, respectively, in good to excellent yields.
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