Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 28, Pages 10250-10253Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja404181c
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Funding
- NSF [DMR-1200451]
- NSFC [NSFC-21271135]
- Soochow University [Q410900712]
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [1200451] Funding Source: National Science Foundation
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We apply a two-step strategy to realize ordered distribution of multiple components in one nanocluster (NC) with a crystallographically ordered core/shell structure. A coreless supertetrahedral chalcogenide Cd-In-S cluster is prepared, and then a copper ion is inserted at its void core site through a diffusion process to form a Cu-Cd-In-S quaternary NC. This intriguing molecular duster with mono-copper core and Cd-In shell exhibits enhanced visible-light-responsive optical and photoelectric properties compared to the parent NC.
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