Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 14, Pages 5286-5289Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja401034g
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Funding
- National Basic Research Program of China (973 Program) [2011CB808600]
- National Nature Science Foundation of China [20932002, 21172076, 21202046]
- Guangdong Natural Science Foundation [10351064101000000, S2012040007088]
- Fundamental Research Funds for the Central Universities [2012ZP0003, 2012ZB0011]
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A novel and efficient palladium-catalyzed dehydrogenative aminohalogenation of alkenes with molecular oxygen as the sole oxidant has been developed. This protocol provides a valuable synthetic tool for the assembly of a wide range of brominated enamines under mild conditions, with unprecedented stereoselectivity and exceptional functional group tolerance. This attractive route for the synthesis of brominated enamines is of great significance due to the products' versatile reactivity for further transformations.
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