Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 25, Pages 9240-9243Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja4042077
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Funding
- Air Force Office of Scientific Research (Young Investigator Award) [FA9550-11-1-0032]
- National Science Foundation [DBI-115269, CHE-1059084]
- European Community [PIOF-GA-2009-252856]
- NSF [OCI-1053575]
- Direct For Mathematical & Physical Scien [1059084] Funding Source: National Science Foundation
- Division Of Chemistry [1059084] Funding Source: National Science Foundation
- Div Of Biological Infrastructure
- Direct For Biological Sciences [1340038] Funding Source: National Science Foundation
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Cyclopentadienes (CPs) with Raman and electrochemically active tags were patterned covalently onto graphene surfaces using force-accelerated Diels-Alder (DA) reactions that were induced by an array of elastomeric tips mounted onto the piezoelectric actuators of an atomic force microscope. These force-accelerated cycloadditions are a feasible route to locally alter the chemical composition of graphene defects and edge sites under ambient atmosphere and temperature over large areas (similar to 1 cm(2)).
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