Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 2, Pages 648-650Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja311796n
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Funding
- Loker Hydrocarbon Research Institute
- United States Department of Energy
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A catalyst based on nickel oxide on magnesium oxide (NiO/MgO) thermally activated under hydrogen is effective for the bi-reforming with steam and CO2 (combined steam and dry reforming) of methane as well as natural gas in a tubular flow reactor at elevated pressures (5-30 atm) and temperatures (800-950 degrees C). By adjusting the CO2-to-steam ratio in the gas feed, the H-2/CO ratio in the produced syn-gas could be easily adjusted in a single step to the desired value of 2 for methanol and hydrocarbon synthesis.
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