Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 34, Pages 13926-13929Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja3043905
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Funding
- AIST
- METI
- US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences
- Grants-in-Aid for Scientific Research [22560768] Funding Source: KAKEN
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Ultrafine Pt nanoparticles were successfully immobilized inside the pores of a metal-organic framework, MIL-101, without aggregation of Pt nanoparticles on the external surfaces of framework by using a double solvents method. TEM and electron tomographic measurements clearly demonstrated the uniform three-dimensional distribution of the ultrafine Pt NPs throughout the interior cavities of MIL-101. The resulting Pt@ MIL-101 composites represent the first highly active MOF-immobilized metal nanocatalysts for catalytic reactions in all three phases: liquid-phase ammonia borane hydrolysis, solid-phase ammonia borane thermal dehydrogenation, and gas-phase CO oxidation.
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