Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 26, Pages 10942-10946Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja303023n
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Funding
- National Institutes of Health [GM099142]
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The tandem ylide formation/[2,3]-sigmatropic rearrangement between donor/acceptor rhodium carbenoids and chiral allyl alcohols is a convergent C-C bond forming process, which generates two vicinal stereogenic centers. Any of the four possible stereoisomers can be selectively synthesized by appropriate combination of the chiral catalyst Rh-2(DOSP)(4) and the chiral alcohol.
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