Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 49, Pages 20001-20004Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja309724w
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- Funding Program for World-Leading Innovative R&D on Science and Technology (FIRST), Japan
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We have established a well-defined dome-shaped T-c curve in Ir0.94-xRhxSe2 superconductors. The maximum T-c(onset) of 9.6 K was obtained at x = 0.36, at which the Se-Se separation in the dimer anion is the longest. Simultaneously, the destabilization of Se-Se dimers accompanied by partial electron transfer from the Ir/Rh to the chalcogenide ions resulted in the emergence of optimal T-c.
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