Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 33, Pages 13773-13779Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja304925t
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Funding
- Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-76-SFO0515]
- U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering
- U.S. Department of Energy by LLNL [DE-AC52-07NA27344]
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We have developed a chemical method to intercalate a variety of zerovalent metal atoms into two-dimensional (2D) layered Bi2Se3 chalcogenide nanoribbons. We use a chemical reaction, such as a disproportionation redox reaction, to generate dilute zerovalent metal atoms in a refluxing solution, which intercalate into the layered Bi2Se3 structure. The zerovalent nature of the intercalant allows superstoichiometric intercalation of metal atoms such as Ag, Au, Co, Cu, Fe, In, Ni, and Sn. We foresee the impact of this methodology in establishing novel fundamental physical behaviors and in possible energy applications.
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