Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 13, Pages 5750-5753Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja300684r
Keywords
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Categories
Funding
- Tekes
- Orion under Tekes
- CABB under Tekes
- Hormos Medical under Tekes
- PCAS Finland under Tekes
- Fermion under Tekes
- Pharmatory under Tekes
- AB Enzymes under Tekes
- Academy of Finland (KR) [130629, 122350, 140718]
- Academy of Finland (AKA) [130629, 140718, 122350, 140718, 122350, 130629] Funding Source: Academy of Finland (AKA)
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The dehydrogenative beta'-functionalization of a-substituted beta-keto esters with indoles proceeds with high regioselectivities (C3-selective for the indole partner and beta'-selective for the beta-keto ester) and good yields under mild palladium catalysis at room temperature with a variety of oxidants. Two possible mechanisms involving either late or early involvement of indole are presented.
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