Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 6, Pages 2860-2863Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja211455j
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Funding
- Schlumberger Foundation's Faculty for the Future
- NRSCC
- University of Amsterdam
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A chiral supramolecular ligand has been assembled and applied to the rhodium-catalyzed asymmetric hydroformylation of unfunctionalized internal alkenes. Spatial confinement of the metal center within a chiral pocket results in reversed regioselectivity and remarkable enantioselectivities.
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