Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 48, Pages 19922-19934Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja310351e
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Funding
- National Institutes of Health [GM46059, 1F32GM088931]
- National Science Foundation [2010094243, CHE 980861, DBI 9729592, CHE 0946721]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [946721] Funding Source: National Science Foundation
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A series of monoligated L.Pd-II(Ar)X complexes (L = dialkyl biaryl phosphine) have been prepared and studied in an effort to better understand an unusual dearomative rearrangement previously documented in these systems. Experimental and theoretical evidence suggest a concerted process involving the unprecedented Pd-II-mediated insertion of an aryl group into an unactivated arene.
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