Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 37, Pages 15265-15268Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja307042z
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Funding
- Ministerio Espanol de Ciencia e Innovacion [CTQ2010-15364, MAT2010-16891, CSD2007-00010, DPI 2010-21103-CO4-O3]
- Generalitat Valenciana [PROMETEO/2009/108, ISIC2012/002]
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Two two-dimensional (2D) systems having the formula [{Fe-III(dmbpy)(CN)(4)}(2)(CoL)-L-II](n) [L = pyetNO (1), tvpNO (2)] and consisting of single-chain magnets connected through organic ligands (L) have been prepared, and their magnetic properties have been investigated. The overall magnetic behavior depends on the capacity of the organic pillars to transmit long-range magnetic interactions. 1 is the first example of a 2D compound exhibiting double relaxation of the magnetization, whereas 2 behaves as a metamagnet.
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