Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 135, Issue 1, Pages 58-61Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja310449k
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- ARC
- Monash University
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The N-heterocyclic carbene (NHC)-catalyzed Claisen rearrangement of hybrid Ireland-Coates structures has been achieved, allowing the stereoselective synthesis of highly functionalized beta-lactones. The reaction proceeds with high diastereoselectivity (>20:1) and affords a diverse range of beta-lactone fused cyclopentanes. Mechanistic studies are detailed.
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