Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 45, Pages 18495-18498Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja307851b
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Funding
- W. W. Caruth, Jr. Endowed Scholarship
- Robert A. Welch Foundation [I-1748]
- American Cancer Society Petroleum Research Fund [51710-DN11]
- National Institutes of Health [1R01GM102604-01]
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The enantioselective allylic am nation. of unactivated terminal olefins represents a direct and attractive strategy for the synthesis of enantioenriched amines. We have developed the first use of a nitrogen. containing reagent and a chiral palladium catalyst to convert unfunctionalized olefins into enantioenriched allylic amines via an ene reaction/[2,3]-rearrangement.
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