Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 134, Issue 12, Pages 5464-5467Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja300003t
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Funding
- Ministry of Science and Technology of China [2010CB631302]
- National Natural Science Foundation of China [51071047, 51133001]
- PhD Programs Foundation of Ministry of Education of China [20110071110009, 20110071130002]
- Science and Technology Commission of Shanghai Municipality [11JC1400700, 11520701100, 10JC1401900]
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The recyclable dehydrogenation of ammonia borane (AB) is achievable within a graphene oxide (GO)-based hybrid nanostructure, in which a combined modification strategy of acid activation and nanoconfinement by GO allows AB to release more than 2 equiv of pure H-2 at temperatures below 100 degrees C. This process yields polyborazylene (PB) as a single product and, thus, promotes the chemical regeneration of AB via reaction of PB with hydrazine in liquid ammonia.
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