Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 133, Issue 6, Pages 1781-1783Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja110870f
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Funding
- National Natural Science Foundation of China [20972027]
- NENU [NENU-STC08013/STB07007]
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An aza-oxy-carbanion relay via tandem Michael addition/ring opening of cyclopropane and recyclization/carbanion migration/electrophile trapping has been developed by the utilization of 1-cinnamoylcyclopro-panecarboxamides to react with various electrophiles. This represents the first example of anion relay chemistry via non-Brook rearrangement. This novel protocol has been applied in the facile and efficient synthesis of biologically active bicyclic furo[3,2-c]pyridinone compounds.
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